The relationship between the natural radioactivity of rocks and soils formed on them – the basic problem of the interpretation of data gathered by airborne and field gamma-ray spectrometry

Vol.22,No.1-2(2015)

Abstract
The objective of this study was to assess the amount of natural radionuclides in fresh parent rocks and their effect on natural radioactivity of soils developed from them. Forty-five fresh rocks consisting mainly of granitoids, syenitoids, acid to basic metavolcanites, mica schists, gneisses, quartzites, serpentinites, sandstones, graywackes, and limestones and their corresponding overlying soils were sampled for laboratory gamma-ray spectrometric analysis. Contents of potassium, uranium and thorium were converted to mass activity of 226Ra equivalent (am) and terrestrial gamma radiation dose rate (D). Data are tabled and discussed. The highest am values occured in syenitoids (386–441 Bq·kg-1) followed by granitoids, mica schists, greywackes and gneisses, whereas the lowest am values were found in quartzose sandstones (15–36 Bq·kg-1) followed by limestones (less than 15 Bq·kg-1) and serpentinites (less than 6 Bq·kg-1). The natural radioactivity of soils is usually slightly lower than that of parent rocks due to the lower content of potassium, uranium and thorium in soils. This is typical for granitoids, syenitoids and rocks of similar mineralogical composition. In soils developed on granitoids and syenitoids were found increased concentrations of all three elements in the grain size fraction below 0.063 mm. Soils developed on rocks with low natural radioactivity (such as limestones and serpentinites) tend to have significantly higher natural radioactivity than their parent rocks. This may complicate the interpretation of data obtained by airborne gamma-ray spectrometry.

Keywords:
soils; rocks; gamma-spectrometry; natural radioactivity; gamma dose rate
References

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